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Yang, K., et al., Role of chiral quantum Hall edge states in nuclear spin polarization. Nat Commun, 2017. 8: p. 15084.
Resistively detected NMR (RDNMR) based on dynamic nuclear polarization (DNP) in a quantum Hall ferromagnet (QHF) is a highly sensitive method for the discovery of fascinating quantum Hall phases; however, the mechanism of this DNP and, in particular, the role of quantum Hall edge states in it are unclear. Here we demonstrate the important but previously unrecognized effect of chiral edge modes on the nuclear spin polarization. A side-by-side comparison of the RDNMR signals from Hall bar and Corbino disk configurations allows us to distinguish the contributions of bulk and edge states to DNP in QHF. The unidirectional current flow along chiral edge states makes the polarization robust to thermal fluctuations at high temperatures and makes it possible to observe a reciprocity principle of the RDNMR response. These findings help us better understand complex NMR responses in QHF, which has important implications for the development of RDNMR techniques.
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Demonstration of open-quantum-system optimal control in dynamic nuclear polarization
From The DNP-NMR Blog:
Demonstration of open-quantum-system optimal control in dynamic nuclear polarization
Sheldon, S. and D.G. Cory, Demonstration of open-quantum-system optimal control in dynamic nuclear polarization. Physical Review A, 2015. 92(4): p. 042102.
http://link.aps.org/doi/10.1103/PhysRevA.92.042102
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01-07-2016 08:36 AM
A high saturation factor in Overhauser DNP with nitroxide derivatives: the role of (14)N nuclear spin relaxation
From The DNP-NMR Blog:
A high saturation factor in Overhauser DNP with nitroxide derivatives: the role of (14)N nuclear spin relaxation
Enkin N, Liu G, Gimenez-Lopez Mdel C, Porfyrakis K, Tkach I, Bennati M. A high saturation factor in Overhauser DNP with nitroxide derivatives: the role of (14)N nuclear spin relaxation. Phys Chem Chem Phys. 2015;17(17):11144-9.
http://www.ncbi.nlm.nih.gov/pubmed/25855020
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05-21-2015 03:46 AM
Dynamic nuclear polarization and Hanle effect in (In,Ga)As/GaAs quantum dots. Role of nuclear spin fluctuations
From The DNP-NMR Blog:
Dynamic nuclear polarization and Hanle effect in (In,Ga)As/GaAs quantum dots. Role of nuclear spin fluctuations
Gerlovin, I.Y., et al., Dynamic nuclear polarization and Hanle effect in (In,Ga)As/GaAs quantum dots. Role of nuclear spin fluctuations. AIP Conference Proceedings, 2013. 1566(1): p. 319-320.
http://scitation.aip.org/content/aip/proceeding/aipcp/10.1063/1.4848414
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12-06-2014 04:54 AM
Dynamic nuclear polarization and Hanle effect in (In,Ga)As/GaAs quantum dots. Role of nuclear spin fluctuations
From The DNP-NMR Blog:
Dynamic nuclear polarization and Hanle effect in (In,Ga)As/GaAs quantum dots. Role of nuclear spin fluctuations
Gerlovin, I.Y., et al., Dynamic nuclear polarization and Hanle effect in (In,Ga)As/GaAs quantum dots. Role of nuclear spin fluctuations. AIP Conference Proceedings, 2013. 1566(1): p. 319-320.
http://scitation.aip.org/content/aip/proceeding/aipcp/10.1063/1.4848414
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11-18-2014 01:39 AM
The role of level anti-crossings in nuclear spin hyperpolarization
The role of level anti-crossings in nuclear spin hyperpolarization
Publication date: August 2014
Source:Progress in Nuclear Magnetic Resonance Spectroscopy, Volume 81</br>
Author(s): Konstantin L. Ivanov , Andrey N. Pravdivtsev , Alexandra V. Yurkovskaya , Hans-Martin Vieth , Robert Kaptein</br>
Nuclear spin hyperpolarization is an important resource for increasing the sensitivity of NMR spectroscopy and MRI. Signal enhancements can be as large as 3–4 orders of magnitude. In hyperpolarization experiments, it is often desirable to transfer the initial...
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08-24-2014 04:05 PM
The role of level anti-crossings in nuclear spin hyperpolarization
From The DNP-NMR Blog:
The role of level anti-crossings in nuclear spin hyperpolarization
Ivanov, K.L., et al., The role of level anti-crossings in nuclear spin hyperpolarization. Prog. NMR. Spec., 2014. 81(0): p. 1-36.
http://www.sciencedirect.com/science/article/pii/S0079656514000454
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08-18-2014 10:14 PM
Role of Electron Spin Dynamics on Solid-State Dynamic Nuclear Polarization Performance
From The DNP-NMR Blog:
Role of Electron Spin Dynamics on Solid-State Dynamic Nuclear Polarization Performance
Siaw, T.A., et al., Role of Electron Spin Dynamics on Solid-State Dynamic Nuclear Polarization Performance. Phys. Chem. Chem. Phys., 2014.
http://dx.doi.org/10.1039/C4CP02013H
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06-20-2014 08:14 PM
Long-lived nuclear spin states in methyl groups and quantum-rotor-induced polarization
From The DNP-NMR Blog:
Long-lived nuclear spin states in methyl groups and quantum-rotor-induced polarization
Meier, B., et al., Long-lived nuclear spin states in methyl groups and quantum-rotor-induced polarization. J Am Chem Soc, 2013. 135(50): p. 18746-9.
http://www.ncbi.nlm.nih.gov/pubmed/24252212